Effect of Morphological Modification over g-C3N4 on Photocatalytic Hydrogen Evolution Performance of g-C3N4-Pt Photocatalysts

نویسندگان

چکیده

In this study, the morphological properties of g-C3N4 in g-C3N4-Pt photocatalysts were modified by a simple hydrothermal treatment for photocatalytic hydrogen evolution. addition, modification effect on evolution performance was investigated. The long-time clearly changed morphology building extended melem units with more oxygen functional groups at defect edges units, which evidenced X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), and photoelectron (XPS) measurements. different features resulted lower photoluminescence (PL) emission intensity PL spectra smaller semicircle radius electrochemical impedance (EIS) data. This indicates efficient charge separation photocatalyst morphology. Consequently, morphologically showed higher rate due to better efficiency.

برای دانلود باید عضویت طلایی داشته باشید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Enhanced Photocatalytic Performance of Luminescent g-C3N4 Photocatalyst in Darkroom.

Graphitic-C3N4(g-C3N4), a low-cost visible-light-driven photocatalyst, was used for the photocatalytic oxidation of aqueous methylene blue (MB) in the dark with Sr4Al14O25:(Eu,Dy) assistance. The Sr4Al14O25:(Eu,Dy)/g-C3N4 photocatalysts were fabricated through the ultrasonic dispersion method. The commercial Sr4Al14O25:(Eu,Dy) phosphor was used as a long afterglow supplier for exciting g-C3N4 i...

متن کامل

Pt‐Decorated g‐C3N4/TiO2 Nanotube Arrays with Enhanced Visible‐Light Photocatalytic Activity for H2 Evolution

Aligned TiO2 nanotube layers (TiNTs) grown by self-organizing anodization of a Ti-substrate in a fluoride-based electrolyte were decorated with graphitic-phase C3N4 (g-C3N4) via a facile chemical vapor deposition approach. In comparison with classical TiO2 nanotubes (anatase), the g-C3N4/TiNTs show an onset of the photocurrent at 2.4 eV (vs. 3.2 eV for anatase) with a considerably high photocur...

متن کامل

Shell-engineering of hollow g-C3N4 nanospheres via copolymerization for photocatalytic hydrogen evolution.

Incorporation of aromatic motifs into the nanosized shells of hollow carbon nitride nanospheres has been reported to develop functional photosynthetic structures for solar energy application. This modification results in an extended π-conjugation system, red-shift of the optical absorption, and an improved charge separation in the shell, while still retaining the unique hollow polymeric nanoarc...

متن کامل

Ti4O7/g-C3N4 Visible Light Photocatalytic Performance on Hypophosphite Oxidation: Effect of Annealing Temperature

The oxidation of hypophosphite to phosphate is the key to recover the phosphorus resource from the hypophosphite wastewater. In the present work, Ti4O7/g-C3N4 composites were synthesized at two different temperatures (100 and 160°C) and their performance on photocatalytic oxidation of hypophosphite under visible light irradiation and the corresponding mechanism were evaluated. A hydrolysis meth...

متن کامل

PtNi Alloy Cocatalyst Modification of Eosin Y-Sensitized g-C3N4/GO Hybrid for Efficient Visible-Light Photocatalytic Hydrogen Evolution

An economic and effective Pt-based alloy cocatalyst has attracted considerable attention due to their excellent catalytic activity and reducing Pt usage. In this study, PtNi alloy cocatalyst was successfully decorated on the g-C3N4/GO hybrid photocatalyst via a facile chemical reduction method. The Eosin Y-sensitized g-C3N4/PtNi/GO-0.5% composite photocatalyst yields about 1.54 and 1178 times h...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Catalysts

سال: 2023

ISSN: ['2073-4344']

DOI: https://doi.org/10.3390/catal13010092